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The Center of Excellence for Stewardship Science is a collaboration between Rutgers
University, UNIRIB/
ORAU with ORNL , Tennessee Technological University,
Colorado School of Mines, University of North Carolina and
the NNSA Lawrence
Livermore and
Los Alamos National Laboratories.The Center is
involved with experiments at the Holifield Radioactive Ion Beam
Facility of Oak Ridge National
Laboratory . The aim of the Center is to provide nuclear structure
input on unstable species of importance to nuclear structure, nuclear astrophysics
and science-based stockpile stewardship.
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| Thomas P. D’Agostino (center) is Deputy
Administrator for Defense Programs in the Department of Energy’s
(DOE) National Nuclear Security Administration (NNSA). Deputy
Administrator D’Agostino leads NNSA’s weapons programs, which
maintain the reliability of our nation’s nuclear weapons stockpile.
Pictured with him at the Stewardship Science Academic Alliance (SSAA)
Symposium held at the Carnegie Intuition in Washington, DC, February
26-28, 2008 are: Cara Jost, ORAU and University of Mainz; Travis
Bray, Auburn University; Kelly Chipps, Colorado School of Mines;
Sean Liddick, University of Tennessee; Steven Padgett, University of
Tennessee; Catalin Matei, ORAU; Patrick O’Malley, Rutgers; William
Peters, Rutgers; Jolie Cizewski, Rutgers.Also attending, but not
pictured, was Ken Carter, (ORAU), Robert Hatarik (Rutgers) and
Steven Pain (ORNL/UT). |
Neutron Transfer Measurements
Single-neutron transfer reactions, such as (d,p), provide information
which is useful for nuclear structure, astrophysics and stewardship
science studies. These reactions, with stable, light ion beams, have been
used for decades to extract information about the spins and parities as
well as single-particle properties of nuclei resulting from reactions of
stable beams on targets of stable or long-lived isotopes. Now
with sufficient Radioactive Ion Beam (RIB) intensities it is possible
to perform (d,p) reactions in inverse kinematics, using a heavy
radioactive species as the beam and a deuterated polyethylene target,
allowing us to study nuclei away from the valley of stability.
At the HRIBF, we use RIBs produced from proton-induced
fission on a uranium carbide target. This production mechanism
supplies many species of neutron-rich nuclei, including those close to
the shell closures at N=50 and N=82. The 25-MV
tandem Van de Graaff accelerator is capable of accelerating beams to around the
Coulomb barrier, a favorable energy regime for transfer reactions.
The protons resulting from the (d,p) reaction are measured in
various silicon detectors including the
SIDAR array and silicon strip detector
telescopes. The beam-like recoil particles are detected in an ion
counter .
The program to date has had a number of successes, including the first spectroscopic
measurement of the r-process nucleus 83Ge and a measurement of another N=51
neutron-rich isotone, 85Se. We have recently performed three (d,p) measurements on nuclei near the double shell closure at 132Sn - 130Sn(d,p) 131Sn, 132Sn(d,p)133Sn and 134Te(d,p)135Te.
Measurements using radioactive beams require efficient detector arrays,
due to the relatively low beam intensities currently obtainable
(compared to stable beams) . The Oak Ridge Rutgers University Barrel
Array (ORRUBA) is a large solid angle silicon detector array, capable of
providing energy, angle and particle identification information. ORRUBA
is comprised of two rings of 12 position-sensitive silicon detector
telescopes, symmetrically covering angles forward and backward of 90
degrees (relative to the target location). Each telescope consists of a
thin (65um or 140um) transmission (dE) detector, and a thick(1000um)
stopping (E) detector, enabling particle identification and measurement
of the energy of particles of interest. Each detector is ~8cm long, and
its width is divided into four 1cm wide resistive strips, oriented
parallel to the beam axis. Readouts from both ends of each strip allow
measurement of the position of the interaction, allowing determination
of the emission angle of the detected particles.
ORRUBA is currently in its design phase. The prototype detectors are being
manufactured by Micron Semiconductors Ltd, and a
new chamber is being constructed to accommodate the array.
(d,p gamma)
The Q-value resolution of (d,p) reactions in inverse kinematics is limited by the kinematic
conditions. However, it is possible to measure the excitation levels of excited states
populated in the reaction, as well as others in the subsequent cascade, using the emitted
gamma-rays.Gamma-ray cascades
also give information on the spin-parities of the states, thus yielding important nuclear structure
information. Tagging on the gamma-rays can help to clarify the proton spectra and reduce background.
As the energy resolution is now independent of the reaction it is possible to use
thicker targets to increase the yield. It is important, at the same time, to use arrays of
high resolution detectors in close geometry.
The Stewardship Collaboration will test the feasibility of (d,p gamma)
measurements at the HRIBF at ORNL. Currently, a chamber is being built to house pre-existing
detection systems such as SIDAR, silicon telescopes and germanium clover detectors. SIDAR,
in the lamp shade configuration, will cover "back angles" between 120 degrees to 160 degrees
in the lab frame. Four silicon telescopes, 5cm by 5cm position sensitive strip detectors,
will cover 90 degrees and back to 120 degrees in the lab frame. Finally, four germanium clovers will
be mounted at 90 degrees in the CARDS configuration. The efficiency of the system is dictated by
the efficiency of the clovers, which is 4% at 1.333 MeV.
The initial test will utilize a stable 88Sr beam. This beam was chosen because of its
close proximity to unstable nuclei of interest to the stewardship center. Radioactive
nuclei in the Sr region will be examined using the proton-gamma coincidence method upon
successful completion of the stable run. In the future the ORRUBA system will be combined
with gamma-ray coincidence capabilities to be used with RIB experiments.

Ion Source Development
Radioactive Ion Beams (RIBs) at the HRIBF are produced via the ISOL method, where a thick target is
bombarded with light ions, such as protons, deuterons or alpha particles. The radioactive species
produced in the reaction has to diffuse out of the production target and is transported to the ion source
where it is ionized and accelerated. These steps are highly dependent on the chemistry of the isotope.
Neutron-rich beams are produced at the HRIBF via the fission of uranium. In this case, isotopes of many
different elements are produced simultaneously. Hence, it is often necessary to perform chemical
separation in addition to mass separation. This chemical separation has to performed in-situ and
on0line by using chemical properties for the element of interest.
Many beam are available at the HRIBF, however in some cases the purity or intensity needs to be improved
before they can be used for transfer reactions. For instance, for some very short lived isotopes, the
time required to extract and transport the ion can be long compared with the nuclear half life, leading
to significant losses in intensity. The RIB development team of the Center of Excellence is working to
understand all the processes which take place in a target-ion source and to optimize each of them in
order to purify beams and increase their intensities. The Center of Excellence is also interested in
experiments on proton-rich isotopes which are relevant to radiochemical detectors for stewardship
science. This involves the development of new beams. Different target materials are under investigation
for fast release of reaction products.
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Jolie
Cizewski,
Principle Investigator, Rutgers University
Ken Carter,
Co-Principle Investigator, ORAU/UNIRIB
Dan Bardayan,
ORNL Staff Member
Jeffrey Blackmon,
ORNL Staff Member
Ryan Fitzgerald,
Graduate Student, University of North Carolina, Chapel Hill
Patty
Gulyas, Secretary, Rutgers University
Micah Johnson,
Post doc, ORAU
Kate Jones,
Post doc, Rutgers University
Ray Kozub,
Professor, Tennessee Technological University
Andreas Kronenberg,
Post doc, ORAU |
Jake
Livesay, Graduate Student, Colorado School of Mines
Zhanwen Ma, Graduate
Student, University of Tennessee
Caroline Nesaraja,
Post doc, ORNL
Steve Pain,
Post doc, Rutgers University
Charles Reed,
Technician, ORAU/UNIRIB
Gene Spejewski,
Consultant, ORAU/UNIRIB
Jeffry Thomas,
Grad Student, Rutgers University
Dale Visser,
Post Doc, University of North Carolina, Chapel Hill
Ally Wright,
Administrative Assistant, ORAU/UNIRIB |
Coming soon.
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